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Modification of the conductance of single fullerene molecules by endohedral doping
Institut für Bio- und Nanosysteme, Forschungszentrum Jülich.
Tyndall National Institute, University College Cork.
Department of Physics, Queen Mary University of London.
Department of Physics, Queen Mary University of London.
Vise andre og tillknytning
2009 (engelsk)Inngår i: Applied Physics Letters, ISSN 0003-6951, E-ISSN 1077-3118, Vol. 95, nr 13Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

We use scanning tunneling microscopy to establish controlled contacts to single molecules of endohedrally doped Ce 2@C 80 fullerenes with C 60 as a reference. The stability of the experimental setup allows for the determination of the conductance of Ce 2@C 80 relative to the conductance of C 60. The endohedral doping reduces the conductance of Ce 2@C 80 by a factor of about five with respect to C 60. Ab initio calculations show that the reason for this reduced conductance is the absence of electron orbitals delocalized over the cage of Ce 2@C 80 in the energy window of the conductance measurement

sted, utgiver, år, opplag, sider
2009. Vol. 95, nr 13
Identifikatorer
URN: urn:nbn:se:ltu:diva-8839DOI: 10.1063/1.3236529Lokal ID: 76349a31-33dc-4142-b8a4-17255c66a95aOAI: oai:DiVA.org:ltu-8839DiVA, id: diva2:981777
Merknad
Upprättat; 2009; Bibliografisk uppgift: Article number 133118; 20130227 (andbra)Tilgjengelig fra: 2016-09-29 Laget: 2016-09-29 Sist oppdatert: 2017-11-24bibliografisk kontrollert

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