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Colloidal processing and CO 2 capture performance of sacrificially templated zeolite monoliths
Department of Materials and Environmental Chemistry, Berzelii Center EXSELENT on Porous Materials, Stockholm University.ORCID-id: 0000-0003-4888-6237
Department of Materials and Environmental Chemistry, Berzelii Center EXSELENT on Porous Materials, Stockholm University.
Department of Materials and Environmental Chemistry, Berzelii Center EXSELENT on Porous Materials, Stockholm University.
Department of Materials and Environmental Chemistry, Berzelii Center EXSELENT on Porous Materials, Stockholm University.
2012 (Engelska)Ingår i: Applied Energy, ISSN 0306-2619, E-ISSN 1872-9118, Vol. 97, s. 289-296Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Sacrificial templating of suspension cast and subsequently thermally treated zeolite monoliths with glassy carbon spheres and fibers yielded zeolite 13X and silicalite-1 monoliths with macroporosities up to 50 vol%. Homogeneous distribution of the macroporosity in hierarchically porous monoliths was obtained by tailoring the surface chemistry of the carbon particles by polyelectrolyte-assisted adsorption of zeolite particles. The effect of amount of kaolin binder and temperature for the thermal treatment on the monoliths strength, surface area and CO2 uptake was studied by diametral compression tests, electron microscopy, X-ray diffraction and gas adsorption. Cyclic adsorption and regeneration measurements showed that zeolite 13X monoliths display a high CO2 uptake while the silicalite-1 monoliths could be regenerated with a relatively low energy penalty.

Ort, förlag, år, upplaga, sidor
2012. Vol. 97, s. 289-296
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Materialteknik
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URN: urn:nbn:se:ltu:diva-39560DOI: 10.1016/j.apenergy.2011.12.064Lokalt ID: e605f840-eafc-43be-8000-069ef49f9912OAI: oai:DiVA.org:ltu-39560DiVA, id: diva2:1013074
Konferens
International Conference on Applied Energy : 16/05/2011 - 18/05/2011
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Upprättat; 2012; 20150416 (farakh); Konferensartikel i tidskriftTillgänglig från: 2016-10-03 Skapad: 2016-10-03 Senast uppdaterad: 2017-11-30Bibliografiskt granskad

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