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Opportunities from Doping of Non-Critical Metal Oxides in Last Generation Light-Conversion Devices
Center for Materials Research, Justus Liebig University Giessen, Heinrich Buff Ring 17, 35392 Giessen, Germany.
Department of Chemical Sciences, University of Padova, via Marzolo 1, Padova, 35131 Italy; Interdepartmental Centre Giorgio Levi Cases for Energy Economics and Technology, University of Padova, via Marzolo 9, Padova, 35131 Italy.
Institute for Microelectronics and Microsystems, Italian National Research Council, Section of Bologna, Bologna, 40129 Italy.
Functional Nanosystems, Italian Institute of Technology, via Morego 30, Genova, 16163 Italy.
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2021 (Engelska)Ingår i: Advanced Energy Materials, ISSN 1614-6832, E-ISSN 1614-6840, Vol. 11, nr 31, artikel-id 2101041Artikel, forskningsöversikt (Refereegranskat) Published
Abstract [en]

The need to develop sustainable energy solutions is an urgent requirement for society, with the additional requirement to limit dependence on critical raw materials, within a virtuous circular economy model. In this framework, it is essential to identify new avenues for light-conversion into clean energy and fuels exploiting largely available materials and green production methods. Metal oxide semiconductors (MOSs) emerge among other species for their remarkable environmental stability, chemical tunability, and optoelectronic properties. MOSs are often key constituents in next generation energy devices, mainly in the role of charge selective layers. Their use as light harvesters is hitherto rather limited, but progressively emerging. One of the key strategies to boost their properties involves doping, that can improve charge mobility, light absorption and tune band structures to maximize charge separation at heterojunctions. In this review, effective methods to dope MOSs and to exploit the derived benefits in relation to performance enhancement in different types of devices are identified and critically compared. The work is focused specifically on the best opportunities coming from the use of non-critical raw materials, so as to contribute in defining an economically feasible roadmap for light conversion technologies based on these highly stable and widely available compounds. 

Ort, förlag, år, upplaga, sidor
John Wiley & Sons, 2021. Vol. 11, nr 31, artikel-id 2101041
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URN: urn:nbn:se:ltu:diva-86289DOI: 10.1002/aenm.202101041ISI: 000669024700001Scopus ID: 2-s2.0-85109140150OAI: oai:DiVA.org:ltu-86289DiVA, id: diva2:1578252
Forskningsfinansiär
EU, Horisont 2020, 101017821EU, Europeiska forskningsrådet, 850875KempestiftelsernaKnut och Alice Wallenbergs Stiftelse
Anmärkning

Validerad;2021;Nivå 2;2021-09-01 (alebob);

Finansiär: Deutsche Forschungsgemeinschaft (101017821, 426888090); Verband der Chemischen Industrie e.V.; DAAD; Interdepartmental Centre Giorgio Levi Cases for Energy Economics and Technology of the University of Padova

Tillgänglig från: 2021-07-06 Skapad: 2021-07-06 Senast uppdaterad: 2021-08-30Bibliografiskt granskad

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Vomiero, Alberto

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