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State to State to State Dynamics of the D+H2→HD+H Reaction: Control of Transition-State Pathways via Reagent Orientation
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China.
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China.
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China.
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China.
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2006 (Engelska)Ingår i: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 96, nr 9, artikel-id 93201Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

The influence of reagent rotation on the dynamics of the D+H2→HD+H reaction is studied. The state-resolved differential cross section is measured using the Rydberg-atom scheme in a crossed beam experiment. It is found that the H2 rotation has a strong influence on the results. This effect was traced to the selection of the quantum bottleneck states through reagent orientation, thus suggesting a novel strategy to control the transition-state pathways in direct chemical reactions.

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2006. Vol. 96, nr 9, artikel-id 93201
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URN: urn:nbn:se:ltu:diva-3210DOI: 10.1103/PhysRevLett.96.093201Lokalt ID: 1023dc4d-77e3-4d51-8958-bd1454ed0df0OAI: oai:DiVA.org:ltu-3210DiVA, id: diva2:976066
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Upprättat; 2006; 20141020 (maggus)Tillgänglig från: 2016-09-29 Skapad: 2016-09-29 Senast uppdaterad: 2017-11-24Bibliografiskt granskad

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