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Spin-orbit and rotational couplings in radiative association of C(3P) and N(4S) atoms
Department of Chemistry and Molecular Biology, University of Gothenburg.
Department of Chemistry, University of Gothenburg.ORCID-id: 0000-0002-7629-0169
Department of Chemistry and Molecular Biology, University of Gothenburg.
2011 (engelsk)Inngår i: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 135, nr 18, artikkel-id 184302Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

The role of spin-orbit and rotational couplings in radiative association of C(3 P) and N(4 S) atoms is investigated. Couplings among doublet electronic states of the CN radical are considered, giving rise to a 6-state model of the process. The solution of the dynamical problem is based on the L2 method, where a complex absorbing potential is added to the Hamiltonian operator in order to treat continuum and bound levels in the same manner. Comparison of the energy-dependent rate coefficients calculated with and without spin-orbit and rotational couplings shows that the couplings have a strong effect on the resonance structure and low-energy baseline of the rate coefficient.

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2011. Vol. 135, nr 18, artikkel-id 184302
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URN: urn:nbn:se:ltu:diva-5462DOI: 10.1063/1.3562125Lokal ID: 390f0873-0808-47fc-9550-88bd2dba7c42OAI: oai:DiVA.org:ltu-5462DiVA, id: diva2:978336
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Upprättat; 2011; 20141018 (maggus)Tilgjengelig fra: 2016-09-29 Laget: 2016-09-29 Sist oppdatert: 2017-11-24bibliografisk kontrollert

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