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Evaluation of value chain configurations for fast pyrolysis of lignocellulosic biomass: Integration, feedstock, and product choice
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Energy Science.ORCID iD: 0000-0002-5662-570x
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Energy Science. International Institute for Applied Systems Analysis (IIASA), Laxenburg, Austria.ORCID iD: 0000-0002-4597-4082
RISE Research Institutes of Sweden, Eklandagatan 86, Göteborg, Sweden.
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Energy Science. International Institute for Applied Systems Analysis (IIASA), Laxenburg, Austria.ORCID iD: 0000-0002-2314-8097
2018 (English)In: Energy, ISSN 0360-5442, E-ISSN 1873-6785, Vol. 144, p. 564-575Article in journal (Refereed) Published
Abstract [en]

Fast pyrolysis of lignocellulosic biomass constitutes a promising technology to reduce dependence on fossil fuels. The product, pyrolysis liquids, can either substitute heavy fuel oil directly, or be upgraded via e.g. hydroprocessing to diesel and petrol. This study presents a systematic evaluation of production costs and CO2 mitigation potentials of different fast pyrolysis value chain configurations. The evaluation considers types of localisations, emissions from electricity and hydrogen production, biomass feedstocks, and final products. The resulting production costs were found to be in the range of 36–60 EUR/MWh for crude pyrolysis liquids, and 61–90 EUR/MWh upgraded to diesel and petrol. Industrial integration was found to be favoured. The CO2 mitigation potential for the pyrolysis liquids was in the range of 187–282 t-CO2/GWh biomass. High variations were found when upgraded to diesel and petrol –best-case scenario resulted in a mitigation of 347 t-CO2/GWh biomass, while worst-case scenarios resulted in net CO2 emissions. Favourable policy support, continued technology development, and/or increased fossil fuel prices are required for the technology to be adapted on an industrial scale. It was concluded that integration with existing industrial infrastructure can contribute to cost reductions and thus help enable the transformation of traditional forest industry into biorefineries.

Place, publisher, year, edition, pages
Elsevier, 2018. Vol. 144, p. 564-575
National Category
Energy Engineering
Research subject
Energy Engineering
Identifiers
URN: urn:nbn:se:ltu:diva-67160DOI: 10.1016/j.energy.2017.12.027ISI: 000425561500046Scopus ID: 2-s2.0-85038946657OAI: oai:DiVA.org:ltu-67160DiVA, id: diva2:1170798
Note

Validerad;2018;Nivå 2;2018-01-04 (svasva)

Available from: 2018-01-04 Created: 2018-01-04 Last updated: 2021-10-15Bibliographically approved
In thesis
1. Forest based biorefinery supply chains - Identification and evaluation of economic, CO2, and resource efficiency
Open this publication in new window or tab >>Forest based biorefinery supply chains - Identification and evaluation of economic, CO2, and resource efficiency
2018 (English)Licentiate thesis, comprehensive summary (Other academic)
Alternative title[sv]
Värdekedjor för skogsbaserade bioraffinaderier – Identifiering och utvärdering av ekonomisk, CO2, och resurseffektivitet
Abstract [en]

Biorefineries for production of fuels, chemicals, or materials, can bean important contribution to reach a fossil-free economy. Large-scaleforest-based biorefineries are not yet cost competitive with their fossil counterparts and it is important to identify biorefinery supply chain configurations with good economic, CO2, and biomass performance if biorefineries are to be a viable alternative to the fossil refineries.

Several factors influence the performance of biorefinery supply chains,e.g. type of conversion process, geographical localisation, and produc-tion capacity. These aspects needs to be analysed in conjunction to identify biorefineries with good supply chain performance. There ares everal approaches to improve the performance of biorefineries, wheree.g. integration with other industries can improve the economic perfor-mance by utilisation of excess heat and by-products. From a Swedish perspective the traditional forest industry is of interest as potential host industries, due to factors such as by-product availability, opportunity for heat integration, proximity to other biomass resources, and their experience in operating large-scale biomass supply chains.

The objectives of this work were to investigate how different supply chain configurations influence the economic, biomass, and CO2 perfor-mance of thermochemical biorefineries integrated with forest industries,as well as methods for evaluating those supply chains.

This work shows that there is an economic benefit for integration with the traditional forest industry for thermochemical biorefineries.This is especially true when the biorefinery concept can replace cur-rent old industrial equipment on site which can significantly improvethe economic performance of the biorefinery, highlighting the role the Swedish forest industry could play to reach a cost efficient large-scale implementation of lignocellulosic biorefineries.

The cost for biomass is a large contributor to the total cost of biore-fineries and for traditional techno-economic evaluations, the biomass prices are considered as static variables. A large-scale biorefinery will likely have an impact on the biomass market, which could lead to both changes in the biomass price, as well as changed biomass demand for other industries. A framework where this is accounted for was intro-duced, combining a techno-economic perspective for evaluating the sup-ply chain performance, with a market model which identifies changes in biomass price and allocation due to the increased biomass competition.

The biorefinery performance can be determined from several per-spectives and system boundaries, both from a plant-level and a national perspective. To facilitate a large-scale introduction of biorefineries and  maximise the benefit from their implementations, there is a need to identify biorefinery concepts with high performance considering severa system boundaries, which has been explored in this work.

Place, publisher, year, edition, pages
Luleå: Luleå University of Technology, 2018
Series
Licentiate thesis / Luleå University of Technology, ISSN 1402-1757
National Category
Bioenergy Energy Engineering
Research subject
Energy Engineering
Identifiers
urn:nbn:se:ltu:diva-67924 (URN)978-91-7790-071-9 (ISBN)978-91-7790-072-6 (ISBN)
Presentation
2018-05-07, Luleå tekniska universitet, Luleå, 10:00 (English)
Opponent
Supervisors
Funder
Swedish Energy Agency
Available from: 2018-03-16 Created: 2018-03-13 Last updated: 2024-03-27Bibliographically approved
2. Evaluation of emerging forest-industry integrated biorefineries: Exploring strategies for robust performance in face of future uncertainties
Open this publication in new window or tab >>Evaluation of emerging forest-industry integrated biorefineries: Exploring strategies for robust performance in face of future uncertainties
2021 (English)Doctoral thesis, comprehensive summary (Other academic)
Abstract [en]

Biorefineries have been promoted to reduce dependency on fossil resources, increase self-sufficiency, and revitalise rural areas. Commercial deployment of forest-based biorefineries has been slow, although academic research has identified several technology options as promising in terms of both costs and resource usage. The low deployment of forest-based biorefinery technologies can be attributed to technology-specific (such as capital cost, process immaturities, and scale-up challenges) or market related (such as biomass and fuel prices, and lack of long-term stable legislation) barriers. The economic and greenhouse gas (GHG) performance of emerging forest-based biorefineries will be highly affected by the assumed characteristics of the surrounding system, such as the assumed energy prices and reference GHG emissions. Future energy prices and policy landscapes are highly uncertain, and, additionally, a successful commercialisation of biorefineries can be expected to have a substantial impact on biomass prices. To fully assess the future performance of emerging biorefinery concepts, these future uncertainties need to be incorporated in the evaluation to identify robust biorefinery concepts that have a high performance for a large set of future market developments. The performance of biorefinery concepts is often assessed using techno-economic approaches, typically using the system boundaries either around the plant, or using a larger geographical area, depending on the scope of the study. The choice of system boundary affects the appropriate methodological choices for the assessment and will depend on the perspective of the evaluation.

This thesis examines the performance of emerging forest industry integrated biorefinery concepts in terms of economy, GHG mitigation potential, and policy support requirement. The aim is to explore strategies to help identify biorefinery concepts with a robust performance considering plant-level design choices and surrounding economic uncertainties. Two perspectives are adopted and compared; i) the performance as seen by a plant-owner, related to the economic performance required for investments to occur, and ii) the performance as seen by a policymaker, related to the cost and impact of implementing the technology on a national level. Biorefinery concepts based on thermochemical conversion technologies are investigated, as they are well suited to a wide variety of residual feedstocks from the forest.

The results show that the production capacity of the biorefinery has a major impact on the economic performance due to economy-of-scale effects. Very large facilities can, from a policymaker perspective, constitute a way to enable a cost-efficient large-scale deployment of biorefineries, while they are not necessary favoured from a plant-owner perspective. This is due to the cost structure of the large-scale deployment of biorefineries, and the division of costs between the plant-owner and other actors in the system.

Traditional techno-economic approaches can be insufficient to identify promising technology configurations considering the wide array of future economic conditions and uncertainties faced by both plant-owners and policymakers. To make any conclusive judgement of the future performance of emerging technologies and investments that can be in operation for more than 20 years, future market developments must be considered. In this thesis, traditional techno-economic analysis is complemented with additional approaches to gain further understanding regarding the future performance of biorefineries. The combined approaches provide complementary insights regarding likely ranges of the future performance depending on future policy ambition levels, as well as impacts of changed biomass prices resulting from the large-scale introduction of biorefineries.

The combined approaches also highlight that, from an economic rationale perspective, policy uncertainty is, in fact, not a major contributor to postponed investments in emerging forest industry-integrated biorefineries. Despite this, the overall results show that most of the examined forest-industry integrated biorefinery concepts would require substantial policy support to become financially viable. A complicating factor is that increased policy support premiering the use of renewable fuels will likely decrease the future prices for the fossil alternatives due to the reduced demand.

This thesis demonstrates that in order to identify robust biorefinery concepts, a multifaceted approach is required to be able to fully capture the interplay between biorefinery configurations and economic performance in face of future uncertainties. Firstly, the plant-owner needs a high probability of a profitable investment; otherwise, investments will not occur. Secondly, for the policymaker, high GHG performance is required, while the cost for large-scale deployment of biorefineries for the entire energy system needs to be kept low. These different objectives can sometimes be at odds with each other, and the policymaker must thus create market incentives that simultaneously premier investments in biorefinery configurations, and benefits the entire energy system.

Place, publisher, year, edition, pages
Luleå: Luleå University of Technology, 2021
Series
Doctoral thesis / Luleå University of Technology 1 jan 1997 → …, ISSN 1402-1544
Keywords
Biorefinery, Biomass, Forest industry, Biofuels, Investment, Gasification, Fast pyrolysis
National Category
Energy Systems
Research subject
Energy Engineering
Identifiers
urn:nbn:se:ltu:diva-84585 (URN)978-91-7790-864-7 (ISBN)978-91-7790-865-4 (ISBN)
Public defence
2021-10-01, E632, Luleå, 10:00 (English)
Opponent
Supervisors
Funder
Swedish Energy Agency, Forskarskolan energisystem
Available from: 2021-05-24 Created: 2021-05-21 Last updated: 2024-04-11Bibliographically approved

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Zetterholm, JonasWetterlund, ElisabethPettersson, KarinLundgren, Joakim

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