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DFT insights into surface properties of anti-perovskite 3D topological crystalline insulators: A case study of (001) surfaces of Ca3SnO
Computational Materials Modeling Laboratory, Department of Physics, Government College University, Faisalabad, 38040, Faisalabad, Pakistan.
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Material Science. Computational Materials Modeling Laboratory, Department of Physics, Government College University, Faisalabad, 38040, Faisalabad, Pakistan.ORCID iD: 0000-0002-8318-214x
Center for Molecular Modeling, Ghent University, 9052 Zwijnaarde, Belgium; Department of Electromechanical, Systems and Metal Engineering, Ghent University, 9052 Zwijnaarde, Belgium; ePotentia, 2600 Antwerp, Belgium.
Department of Physics, Government College Women University, Faisalabad, Faisalabad, Pakistan.
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2021 (English)In: Physics Letters A, ISSN 0375-9601, E-ISSN 1873-2429, Vol. 408, article id 127469Article in journal (Refereed) Published
Abstract [en]

In this letter density functional theory calculations are used for investigating the structural, energetic and electronic properties of CaSn- and Ca2O-terminated (001) surfaces of anti-perovskite Ca3SnO. Our calculations indicate larger structural changes in case of the CaSn-terminated (001) surface of Ca3SnO, however, both CaSn- and Ca2O-terminated surfaces of Ca3SnO are found to be energetically stable. The electronic properties of (001) surfaces of Ca3SnO are examined by taking spin-orbit coupling into account. Comparison of the simulated results of electronic properties for the two (001) surfaces of Ca3SnO with experimentally reported hole carrier densities observed in p-type polycrystalline samples show good agreement.

Place, publisher, year, edition, pages
Elsevier, 2021. Vol. 408, article id 127469
Keywords [en]
Inverse-perovskite, Topological insulator, Surface electronic phenomena, Density functional calculations
National Category
Condensed Matter Physics
Research subject
Applied Physics
Identifiers
URN: urn:nbn:se:ltu:diva-85094DOI: 10.1016/j.physleta.2021.127469ISI: 000658809700001Scopus ID: 2-s2.0-85107414900OAI: oai:DiVA.org:ltu-85094DiVA, id: diva2:1562329
Funder
Knut and Alice Wallenberg FoundationThe Kempe FoundationsSwedish Research Council, 2018-05973
Note

Validerad;2021;Nivå 2;2021-06-09 (alebob);

Finansiär: Higher Education Commission of Pakistan (7107/Punjab/NRPU/R&D/HEC/2017); “Research Centre of Female Scientific and Medical Colleges”, Deanship of Scientific Research, King Saud University

Available from: 2021-06-08 Created: 2021-06-08 Last updated: 2021-06-14Bibliographically approved

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Alay-e-Abbas, Syed Muhammad

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