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Novel Intrinsic Self-Healing Poly-Silicone-Urea with Super-Low Ice Adhesion Strength
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Machine Elements.ORCID iD: 0000-0003-0477-7063
College of Science, Nanjing Forestry University, Nanjing 210037, P. R. China.
Herbert Gleiter Institute of Nanoscience, School of Materials Science and Engineering, Nanjing University of Science and Technology, Nanjing 210037, P. R. China.
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Machine Elements.ORCID iD: 0000-0003-3157-4632
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2022 (English)In: Small, ISSN 1613-6810, E-ISSN 1613-6829, Vol. 18, no 22, article id 2200532Article in journal (Refereed) Published
Abstract [en]

Accumulation of snow and ice often causes problems and even dangerous situations for both industry and the general population. Passive de-icing technologies, e.g., hydrophobic, liquid-infused bionic surfaces, have attracted more and more attention compared with active de-icing technologies, e.g., electric heating, hot air heating, due to the passive de-icing technology's lower energy consumption and sustainability footprint. Using passive de-icing coatings seems to be one of the most promising solutions. However, the previously reported de-icing coatings suffer from high ice adhesion strength or short service life caused by wear. An intrinsic self-healing material based on poly-silicone-urea is developed in this work to address these problems. The material is prepared by introducing dynamic disulfide bonds into the hard phase of the polymer. Experimental results indicate that this poly-silicone-urea has a self-healing efficiency of close to 99%. More interestingly, it is found that the coating prepared from this poly-silicone-urea has a super low ice adhesion force, only 7 ± 1 kPa, which is almost the lowest value compared with previous intrinsic self-healing de-/anti-icing reports. This material can maintain low ice adhesion strength after healing. This intrinsic self-healing poly-silicone-urea can meet several practical applications, opening the door for future sustainable anti-/de-icing technologies.

Place, publisher, year, edition, pages
John Wiley & Sons, 2022. Vol. 18, no 22, article id 2200532
National Category
Manufacturing, Surface and Joining Technology Tribology (Interacting Surfaces including Friction, Lubrication and Wear)
Research subject
Machine Elements
Identifiers
URN: urn:nbn:se:ltu:diva-89955DOI: 10.1002/smll.202200532ISI: 000778739700001PubMedID: 35318812Scopus ID: 2-s2.0-85126871425OAI: oai:DiVA.org:ltu-89955DiVA, id: diva2:1648268
Funder
Swedish Research Council Formas, 2019-00904Swedish Research Council, 2017-04914, 2019-04941Swedish Energy Agency, 2018-003910Interreg Nord, 20202472
Note

Validerad;2022;Nivå 2;2022-06-07 (joosat);

Available from: 2022-03-30 Created: 2022-03-30 Last updated: 2023-09-05Bibliographically approved

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Chen, JunMarklund, PärBjörling, MarcusShi, Yijun

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Manufacturing, Surface and Joining TechnologyTribology (Interacting Surfaces including Friction, Lubrication and Wear)

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