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Mineralization of Trace Nitro/Chloro/Methyl/Amino-Aromatic Contaminants in Wastewaters by Advanced Oxidation Processes
State Key Laboratory of Materials-Oriented Chemical Engineering, Nanjing University of Technology.
State Key Laboratory of Materials-Oriented Chemical Engineering, Nanjing University of Technology.
State Key Laboratory of Materials-Oriented Chemical Engineering, Nanjing University of Technology.
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2010 (English)In: Industrial & Engineering Chemistry Research, ISSN 0888-5885, E-ISSN 1520-5045, Vol. 49, no 13, p. 6243-6249Article in journal (Refereed) Published
Abstract [en]

It has great significance to investigate the degradation of aromatic contaminants as they are highly carcinogenic and nondegradable pollutants in drinking water. In this paper, the mineralization orders of the representative nitro/chloro/methyl/amino-aromatic contaminants with oxidants (OH, H2O2, O-, O2,O3) in advanced oxidation processes (AOPs) are investigated based on the calculated standard molar Gibbs free energy changes of reaction (ΔrGm0) and the results are consistent with those from previous experimental results, electrophilic substitution orientation rules of the Hammett equation, and predicted results with a quantitative structure-activity relationship (QSAR). In addition, the quantitative function relationship between the degradation rate (r) of the aromatic contaminants and the thermodynamic driving force (ΔrGm0) is analyzed in order to investigate the degradation kinetics more rigorously.

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2010. Vol. 49, no 13, p. 6243-6249
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URN: urn:nbn:se:ltu:diva-2552DOI: 10.1021/ie100116cLocal ID: 02c4bea0-fd55-11df-8b95-000ea68e967bOAI: oai:DiVA.org:ltu-2552DiVA, id: diva2:975405
Note
Upprättat; 2010; 20101201 (andbra)Available from: 2016-09-29 Created: 2016-09-29 Last updated: 2017-11-24Bibliographically approved

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Ji, Yuanhui

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