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Electrostatic ordering of the lanthanum endoatom in La@C 82 adsorbed on metal surfaces
Nanoscience Centre, University of Cambridge.
Nanoscience Centre, University of Cambridge.
Tyndall National Institute, University College Cork.
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2005 (English)In: Physical Review B. Condensed Matter and Materials Physics, ISSN 1098-0121, E-ISSN 1550-235X, Vol. 71, no 4Article in journal (Refereed) Published
Abstract [en]

An investigation of the dynamic behavior of the endohedral La atom in La@C 82 adsorbed on Ag(111) or Cu(111) using the normal-incidence x-ray standing wavefield (NIXSW) technique is presented. For the surface-normal (111) reflection, NIXSW demonstrates different La absorption profiles between the La@C 82 monolayer and multilayer. Analysis of the profiles reveals significant La ordering in the monolayer; the degree of ordering increases as the film is cooled. First-principles calculations provide a description of the endohedral metal atom-cage bonding and the fullerene-surface interaction. Combined, these effects give rise to preferential binding sites for the endoatom resulting from electrostatic interactions within the adsorbed fullerene

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2005. Vol. 71, no 4
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URN: urn:nbn:se:ltu:diva-3460DOI: 10.1103/PhysRevB.71.045419Local ID: 1494637a-2498-4424-b132-54e590e3fd4cOAI: oai:DiVA.org:ltu-3460DiVA, id: diva2:976318
Note
Upprättat; 2005; Bibliografisk uppgift: Article number 045419; 20130302 (andbra)Available from: 2016-09-29 Created: 2016-09-29 Last updated: 2017-11-24Bibliographically approved

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