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  • 1.
    Bagheri, Marzieh
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Integrated sewage sludge treatment scenarios – techno-economic analysis on energy and phosphorus recovery2022Licentiatavhandling, sammanläggning (Övrigt vetenskapligt)
    Abstract [en]

    Sewage sludge is a by-product of wastewater treatment that simultaneously gathers contaminants, valuable organic matter, and nutrients. The treatment of the increasing amount of sewage sludge is important from both pollution prevention and resource recovery perspectives as i) large shares of mineral phosphorus, listed as a critical raw material, terminate in the sewage sludge, and ii) energy recovery from sewage sludge can cover the energy-intensive demand of the treatment process. Previous research has identified sewage sludge combustion as a suitable treatment approach as it both addresses contaminant destruction and paves the way for efficient phosphorus recovery from the sewage sludge ash. The commercial development of this practice has, however, been slow. Therefore, this thesis aims to investigate the challenges in sustainable sewage sludge management, and to, in more detail, identify the economic viability of energy and phosphorus recovery from sewage sludge through combustion.

    The thesis’ aim is divided into two objectives addressed in three papers. First, to investigate how different aspects of sewage sludge management, such as contaminants, economic efficiency, technical aspects, and legislation, evolve and interact. This has been done by a review of sewage sludge management research over fifty years (Paper I). Second, to investigate the economic viability of simultaneous energy and phosphorus recovery from sewage sludge by comparing different technology and market scenarios. This has been done for i) new sewage sludge mono-/co-combustion plants (Paper II), and ii) the integration of treatment technologies, mainly anaerobic digestion, hydrothermal carbonization, and combustion, in an existing wastewater treatment plant (Paper III). 

    Results from the analysis of sewage sludge management research (Paper I) show a narrow-focused perspective that often excludes inseparable aspects such as combination of economic consideration and advanced extraction technology. The investment viability of a new mono-/co-combustion of sewage sludge (Paper II) is highly conditional on heat, electricity, and fertilizer price, and external financial support is often a crucial requirement. Sewage sludge co-combustion with potassium-rich biomasses improves sewage sludge quality and forms usable ash as fertilizer without further need for phosphorus recovery technology. In this case, the economic feasibility of the process is independent of usable ash revenue, which stimulates a competitive selling price for the ash, thereby improving the marketing of sludge-based fertilizer. Avoided disposal costs of sewage sludge for a retrofitted wastewater treatment plant by introducing hydrothermal carbonization (Paper III) shows good economic feasibility while recovering phosphorus. Integrating anaerobic digestion, hydrothermal carbonization, and combustion may also improve investment incentives by improving energy outputs and phosphorus recovery. The economic feasibility is contingent on product (hydrochar, heat, electricity) prices and sensitive to added equipment costs, and costs for sludge transportation and disposal. 

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  • 2.
    Bagheri, Marzieh
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Sewage Sludge Treatment Scenarios: Techno-Economic Analyses of Energy and Phosphorus Recovery Focusing on Implementation Challenges2024Doktorsavhandling, sammanläggning (Övrigt vetenskapligt)
    Abstract [en]

    Managing sewage sludge, an inevitable by-product of wastewater treatment processes rich in both contaminants and valuable resources, presents a dual challenge: ensuring pollution prevention by immobilizing or destroying contaminants, and facilitating resource recovery. Balancing these objectives is critical given the growing volumes of sewage sludge and the imperative to both protect the environment and recover valuable resources. The unknown risks of land application of sludge, the currently most common disposal method, make thermal conversion a promising alternative, as it enables energy recovery, the breakdown of potentially harmful organic compounds, and the formation of volume-reduced, sanitized products. Despite the technical feasibility, the commercial development of advanced recovery technologies has been slow. 

    This thesis aims to expand knowledge on different sewage sludge treatment and disposal scenarios under varying conditions; thereby shedding light on implementation challenges, local opportunities, and the financial dynamics critical for phosphorus and energy recovery from the perspectives of wastewater treatment plants, investors, and policymakers. The aim is primarily addressed by performing techno-economic analysis of sewage sludge treatment scenarios, covering the entire sludge treatment process from sludge treatment to end products and disposal (Paper II-V). The techno-economic analysis is supplemented by a review of academic research on sewage sludge management from 1971 to 2019 (Paper I). 

    Results from the analysis of sewage sludge management research (Paper I) show a narrow-focused perspective that often misses the broader, interconnected aspects of sewage sludge management, leading to research that, while detailed, fails to capture the complexity of the field. The investment viability of a new mono-/co-combustion plant for sewage sludge (Paper II) is highly conditional on heat, electricity, and fertilizer prices, and external financial support is often a crucial requirement. Cocombustion of sludge (in low ratios) with K-rich agricultural biomass requirement in and energy demand of a thermal dryer, and by yielding ash that contains phosphorus in a plant-available form. Utilizing existing heat facility (Paper III) and co-combustion to mitigate investment costs and energy demand in sludge management showed the potential to offer a cost-effective alternative to land application. However, the viability of co-combustion hinges on both a high heat market price (Paper II) and the proximity of affordable biomass resources (Paper III). Without these conditions, co-combustion may increase the financial burden of sludge management on wastewater treatment plants and policymakers. 

    Retrofitting a wastewater treatment plant by integrating hydrothermal carbonization in sludge treatment (Paper IV), demonstrated good economic feasibility, primarily due to the avoided disposal costs, while also recovering phosphorus. However, integrating hydrothermal carbonization in a system designed for a thermal dryer may cause a significant reduction in electricity production.

    Given the high moisture content of sludge and the low market prices for fertilizer, the potential revenue from energy and phosphorus recovery is inadequate to solely drive investment in advanced sewage sludge treatment technologies (Papers II-V). This issue is exacerbated by the fact that most wastewater treatment plants are small in scale. Collaborative sludge management across neighboring wastewater treatment plants (Paper V) increases phosphorus recovery capacity and leverages economies of scale, fostering investment in advanced technology. This strategy presents a significant opportunity to lower the treatment costs and offers a competitive alternative to land application, while encompassing energy and phosphorus recovery into the sludge treatment.

    In conclusion, resource recovery and pollution prevention in sludge management is a complex task that necessitates simultaneous consideration of technical aspects, product quality, site-specific conditions, and profitability to ensure a comprehensive and viable approach. Leveraging local infrastructure and resources in sewage sludge management is crucial, highlighting the ecessity for strategies to be tailored to the local opportunities and limitations. Such an approach outperforms mono-combustion by eliminating the investment ensures that solutions are not only environmentally sustainable but also economically viable and socially acceptable. 

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  • 3.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Bauer, Torben
    Luleå tekniska universitet, Institutionen för samhällsbyggnad och naturresurser, Geovetenskap och miljöteknik.
    Ekman Burgman, Linus
    Department of Thematic Studies, Technology and Social Change at Linköping University, 58183, Linköping, Sweden.
    Wetterlund, Elisabeth
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Fifty years of sewage sludge management research: Mapping researchers' motivations and concerns2023Ingår i: Journal of Environmental Management, ISSN 0301-4797, E-ISSN 1095-8630, Vol. 325, artikel-id 116412Artikel i tidskrift (Refereegranskat)
    Abstract [en]

    Sewage sludge management is torn between a desire for pollution prevention and reuse of a valuable resource. Reconciling these interests in sustainable management is a challenge for researchers. This study focuses on how research on sewage sludge management practices has evolved and scrutinizes how this research is interlinked with concerns and societal issues such as contaminants, economic efficiency, and legislation. Based on published academic papers on sewage sludge management between 1971 and 2019, this study found four trends in research focused on sewage sludge management: a decreasing interest in disposal (landfilling and sea dumping), a dominant interest in land application, a growing interest in sewage sludge as product, and a stable interest in energy recovery. Research on disposal focuses on increasing sludge volumes, legislative changes, and economic challenges with an interest in waste co-treatment. Research on land application concerns nutrient use and contaminants, mainly heavy metals. Research on sewage sludge as a product focuses on the extraction of certain resources and less on use of sewage sludge specifically. Research on energy recovery of sewage sludge focuses on volume reduction rather than contaminants. Two-thirds of the papers are detailed studies aiming to improve single technologies and assessing single risks or benefits. As management of sewage sludge is multifaceted, the narrow focus resulting from detailed studies promotes some concerns while excluding others. Therefore, this study highlights potential gaps such as the combination of nutrient use and disposal and energy recovery and nutrient use. 

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  • 4.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap. Energy, Climate and Environment Program, Pollution Management Research Group, International Institute for Applied Systems Analysis - IIASA, Laxenburg, Austria.
    Gómez-Sanabria, Adriana
    Energy, Climate and Environment Program, Pollution Management Research Group, International Institute for Applied Systems Analysis - IIASA, Laxenburg, Austria.
    Höglund-Isaksson, Lena
    Energy, Climate and Environment Program, Pollution Management Research Group, International Institute for Applied Systems Analysis - IIASA, Laxenburg, Austria.
    Economic feasibility and direct greenhouse gas emissions from different phosphorus recovery methods in Swedish wastewater treatment plants2024Ingår i: Sustainable Production and Consumption, ISSN 2352-5509, Vol. 49, s. 462-473Artikel i tidskrift (Refereegranskat)
    Abstract [en]

    Phosphorus (P) is a finite, non-renewable resource that is a critical component of fertilizers; therefore, recovering P from municipal wastewater can provide an alternative sustainable source of this nutrient. This work analyses economic impacts and greenhouse gas emissions of P recovery in Swedish municipal wastewater treatment plants. The study examines different scenarios, including P recovery technologies in individual plants and hubs, and considers various P-rich streams (supernatant, sludge, and ash) in plants, different plant sizes, and multiple sludge management strategies such as land application, incineration, and hydrochar production, under current market conditions. The goal is to identify and offer solutions tailored to local conditions, addressing both technical opportunities and strategies to reduce costs.

    The results show varying recovery rates: 5 % from supernatant, 36–65 % from sludge, and 17 % from sludge ash relative to total P in wastewater. Despite technical feasibility, P recovery costs are not covered at current market prices of P, indicating a lack of financial incentive, especially for smaller treatment plants. The least expensive recovery method costs about 7 k€/t P for ash, compared to 30–187 k€/t P for supernatant, however with the latter coming with the co-benefit of mitigated greenhouse gas emissions. The emissions from studied plants range from 84 to 123 kt CO2 eq (CO2 equivalent) for supernatant, 94–141 kt CO2 eq for sludge, and 75–102 kt CO2 eq for ash among different P recovery methods. Comparatively, P recovery methods from supernatant showed the lowest emissions, while the lower emissions range for ash is due to the consideration of fewer plants. Developing hub networks and converting sludge into products like hydrochar are crucial for attracting investments, enhancing P recovery, and leveraging economies of scale. Results highlight the urgency for localized strategies and proactive policy interventions to reconcile economic and environmental objectives in P recycling. Furthermore, P recovery from wastewater treatment plants, although more resource-intensive than mineral fertilizer, promotes circularity in the food chain and mitigates the risk of eutrophication.

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  • 5.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Gómez-Sanabria, Adriana
    Energy, Climate and Environment Program, Pollution Management Research Group, International Institute for Applied Systems Analysis - IIASA, Laxenburg, Austria.
    Höglund-Isaksson, Lena
    Energy, Climate and Environment Program, Pollution Management Research Group, International Institute for Applied Systems Analysis - IIASA, Laxenburg, Austria.
    Economic feasibility and environmental impacts of phosphorus recovery in Swedish wastewater treatment plantsManuskript (preprint) (Övrigt vetenskapligt)
  • 6.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Wetterlund, Elisabeth
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Introducing hydrothermal carbonization to sewage sludge treatment systems—a way of improving energy recovery and economic performance?2023Ingår i: Waste Management, ISSN 0956-053X, E-ISSN 1879-2456, Vol. 170, s. 131-143Artikel i tidskrift (Refereegranskat)
    Abstract [en]

    Hydrothermal carbonization (HTC) can mitigate the disposal costs of sewage sludge in a wastewater treatment plant. This study analyzes the impact of integrating HTC with anaerobic digestion (AD) and combustion from a combined energy and economic performance perspective. Net energy balance and investment opportunity are investigated for a number of technical scenarios considering i) different combinations of the technologies: AD + HTC, AD + thermal dryer + combustion, and AD + HTC + combustion, ii) different options for HTC process water treatment: wet oxidation (WO) + AD, and direct return to AD, and iii) different products: heat-only, heat and electricity, hydrochar, and phosphorus.

    The results show trade-offs between investment cost, self-supplement of heat, and output electricity when WO is used. In AD + HTC, net heat output decreases compared to the reference plant, but avoided disposal costs and hydrochar revenue result in profitable investment when the process water is directly returned to the AD. Although HTC has a lower heat demand than the thermal dryer, replacing the thermal dryer with HTC is only possible when AD, HTC, and combustion are connected, or when WO covers HTC’s heat demand. HTC may impair the electricity production because of the necessity for a high-temperature heat source, whereas the thermal dryer can utilize a low-temperature heat source. In conclusion, energy advantages of HTC in AD + HTC + combustion are insufficient to provide a promising investment opportunity due to high investment costs of HTC. The investment opportunity improves by co-combustion of hydrochar and external sludge.

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  • 7.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Öhman, Marcus
    Wetterlund, Elisabeth
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Economic viability of co-combusting sewage sludge with agricultural biomasses: a resource-efficient strategy for sludge treatment and phosphorus recovery in SwedenManuskript (preprint) (Övrigt vetenskapligt)
  • 8.
    Bagheri, Marzieh
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Öhman, Marcus
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Wetterlund, Elisabeth
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Techno-Economic Analysis of Scenarios on Energy and Phosphorus Recovery from Mono- and Co-Combustion of Municipal Sewage Sludge2022Ingår i: Sustainability, E-ISSN 2071-1050, Vol. 14, nr 5, artikel-id 2603Artikel i tidskrift (Refereegranskat)
    Abstract [en]

    This study evaluates the techno-economic feasibility of energy and phosphorus (P) fertilizer (PF) recovery from municipal sewage sludge (MSS) through incineration in new combustion plants. We evaluated the economic impact of five critical process design choices: (1) boiler type, (2) fuel (MSS mono-combustion/co-combustion with wheat straw), (3) production scale (10/100 MW), (4) products (heat, electricity, PF), and (5) ash destination. Aspen Plus modeling provided mass and energy balances of each technology scenario. The economic feasibility was evaluated by calculating the minimum selling price of the products, as well as the MSS gate fees required to reach profitability. The dependency on key boundary conditions (operating time, market prices, policy support) was also evaluated. The results showed a significant dependency on both energy and fertilizer market prices and on financial support in the form of an MSS gate fee. Heat was preferred over combined heat and power (CHP), which was feasible only on the largest scale (100 MW) at maximum annual operating time (8000 h/y). Co-combustion showed lower heat recovery cost (19–30 €/MWh) than mono-combustion (29–66 €/MWh) due to 25–35% lower energy demand and 17–25% higher fuel heating value. Co-combustion also showed promising performance for P recovery, as PF could be recovered without ash post-treatment and sold at a competitive price, and co-combustion could be applicable also in smaller cities. When implementing ash post-treatment, the final cost of ash-based PF was more than four times the price of commercial PF. In conclusion, investment in a new combustion plant for MSS treatment appears conditional to gate fees unless the boundary conditions would change significantly.

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  • 9.
    Wetterlund, Elisabeth
    et al.
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Andreas, Lale
    Luleå tekniska universitet, Institutionen för samhällsbyggnad och naturresurser, Geovetenskap och miljöteknik.
    Bagheri, Marzieh
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Bauer, Torben
    Lumire, Sweden.
    Falk, Joel
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Hannl, Thomas Karl
    BEST - Bioenergy and Sustainable Technologies GmbH, Germany.
    Häggström, Gustav
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Johansson, Oskar
    Luleå tekniska universitet, Institutionen för ekonomi, teknik, konst och samhälle, Samhällsvetenskap.
    Lagerkvist, Anders
    Luleå tekniska universitet, Institutionen för samhällsbyggnad och naturresurser, Geovetenskap och miljöteknik.
    Niero, Luisa
    Xylem Water Solutions Sweden, Sweden.
    Pettersson, Maria
    Luleå tekniska universitet, Institutionen för ekonomi, teknik, konst och samhälle, Samhällsvetenskap.
    Söderholm, Patrik
    Luleå tekniska universitet, Institutionen för ekonomi, teknik, konst och samhälle, Samhällsvetenskap.
    Öhman, Marcus
    Luleå tekniska universitet, Institutionen för teknikvetenskap och matematik, Energivetenskap.
    Smart Waste Treatment in the Circular Economy2024Rapport (Övrig (populärvetenskap, debatt, mm))
    Abstract [en]

    This project has targeted utilisation of infrastructure for organic waste treatment in Sweden, in particular sewage sludge, to achieve increased production of high-value materials and energy carriers, reduced use of primary resources, and improved economic performance. We have investigated the sewage sludge management system as a socio-technical system facing a change, with integral connections to the energy and waste systems.

    In conclusion, there is no silver bullet for the future of sewage sludge management. Indeed, it would have to be a full clip of silver bullets, as we found that a mishmash of different barriers –technical, economic, legal, and related to public perception – creates uncertainty that hinders progress regarding both sustainable long-term strategies and technological advancement. The Swedish sewage sludge management is largely fragmented, highlighting the need to shift directionto a more holistic approach. This can help actors address common issues rather than focussing solely on activity-specific problems. Introducing new legislation could be a key step, as the current specific legislation on sewage sludge has a seemingly insignificant role for today’s sludge management, compared to other legislation and the voluntary certification.

    We have formulated six overall research highlights, to outline both published results and meta-conclusions based on combined insights. Each highlight is described separately in this report.

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