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Metal enrichment of soils in three urban drainage grass swales used for seasonal snow storage
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0001-7445-0870
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0003-0367-3449
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0002-4732-7348
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0001-9938-8217
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2021 (English)In: Science of the Total Environment, ISSN 0048-9697, E-ISSN 1879-1026, Vol. 760, article id 144136Article in journal (Refereed) Published
Abstract [en]

Enrichment of soils in three urban drainage swales by metals associated with traffic sources was investigated in a cool temperate climate with seasonal snow. Such swales differed from those not exposed to snow by receiving additional pollutant loads from winter road maintenance involving applications of salt and grit, use of studded tires, and storage and melting of polluted snow cleared from trafficked areas into swales. Among the swales studied, swale L2 in the downtown was the oldest (built around 1960), drained runoff from a road with the highest traffic intensity, and exhibited the highest mean concentrations of most of the metals studied (Pb, Cu, Zn, Cr, Cd, Ni, Co, V, Ti, and W). In the case of Pb, this exceedance was about an order of magnitude: 71 mg/kg DW in L2, compared to about ~8 mg/kg DW in L1 and L3, both built in 1979. Among the metals originating from local geology, barium (Ba) was found in the swales and the grit material at high concentrations of ~650 mg/kg DW and 700–1000 mg/kg DW, respectively. Such concentrations exceeded the Swedish EPA guideline limits of 300 mg/kg DW for less sensitive soil use. The sequential extraction analysis of samples from swale L2 indicated that Ba was mostly in the immobile residual fraction (90%). The absence of clear decline in metal concentrations with distance from the trafficked surfaces suggested that stored snow was another source of metals partly balancing spatial distribution of metals in swale soils.

Place, publisher, year, edition, pages
Elsevier, 2021. Vol. 760, article id 144136
Keywords [en]
Grass swales, Stormwater infiltration, Soil quality, Heavy metals, Sequential extraction
National Category
Water Engineering
Research subject
Urban Water Engineering; Centre - Centre for Stormwater Management (DRIZZLE)
Identifiers
URN: urn:nbn:se:ltu:diva-81133DOI: 10.1016/j.scitotenv.2020.144136ISI: 000607779400139PubMedID: 33341620Scopus ID: 2-s2.0-85098462526OAI: oai:DiVA.org:ltu-81133DiVA, id: diva2:1476485
Funder
Swedish Research Council Formas, 2015–778Vinnova, 2016-05176
Note

Validerad;2021;Nivå 2;2021-01-12 (alebob);

Full text license: CC BY

Available from: 2020-10-14 Created: 2020-10-14 Last updated: 2025-10-22Bibliographically approved
In thesis
1. Trace metals in swale soils and sediments from gully pots and stormwater management ponds
Open this publication in new window or tab >>Trace metals in swale soils and sediments from gully pots and stormwater management ponds
2023 (English)Doctoral thesis, comprehensive summary (Other academic)
Alternative title[sv]
Spårmetaller ackumulerade i dagvattenanläggningar: svackdiken, rännstensbrunnar och dagvattendammar
Abstract [en]

Three commonly used drainage system components, with considerably different characteristics and roles in stormwater management, were studied and reported on in this thesis: (i) grass swales, (ii) gully pots (GPs), and (iii) stormwater management ponds. With time, solids and associated pollutants accumulate in these components, and regular maintenance is needed to ensure that their design functions, including protection of the environment, are sustained.

Trace metals and their concentrations, loads and speciation were investigated within and among the individual types of components. The study program started with a critical review of processes enhancing the quality of stormwater passing over grass filter strips and through swales, and continued with field research of swale soils, and sediments from GPs and ponds.

The swales studied in the thesis served for stormwater drainage and storage of snow cleared from adjacent trafficked areas during winter months. Results suggest that both stormwater runoff and snow stored in the swale were transport vectors of metals originating from traffic. Other sources of metals were native soils and traction material used in winter road maintenance.

Moreover, the speciation results showed that across components, Zn and Pb were the metals with the highest share in the most mobile fraction, followed by Cu, while Ba, Cr,V, Co, and Ni were found in a higher share in the less mobile fractions.

GP and pond sediments showed similar organic matter content, whereas swales soils showed relatively low organic content, further decreasing with the soil depth. Results suggested that higher organic matter content corresponded to higher concentrations of certain metals in the case of ponds and, to some extent, swales. In the case of GPs, a positive relationship between metals and the proportion of fine particles was detected.

The highest concentrations of Cu and Zn were observed in sediments from ponds and reached 319 and 1380 mg/kg DW, respectively. The highest concentration of Pb (188mg/kg DW) was observed in swale, operating for 57 years located next to a road with the traffic intensity of 11,650 v/day.

The large variation in the accumulated dry mass of solids in GPs (2-91 kg) questions the current practice of emptying all GPs at the same regular intervals. Moreover, of the 26 GP samples, Swedish thresholds for soils with the sensitive (S) land use were exceeded for Cu in five samples and Zn in six samples. Of 32 pond samples, the S threshold was exceeded for Cu in nine samples and Zn in 12 samples; of these, three and eight of the pond samples also exceeded the less sensitive (LS) threshold. Of 96 swale samples, 25 samples exceeded the S threshold for Pb, with one sample also exceeding the LS threshold.

Place, publisher, year, edition, pages
Luleå: Luleå University of Technology, 2023
Series
Doctoral thesis / Luleå University of Technology, ISSN 1402-1544
National Category
Water Engineering
Research subject
Urban Water Engineering; Centre - Centre for Stormwater Management (DRIZZLE)
Identifiers
urn:nbn:se:ltu:diva-101706 (URN)978-91-8048-412-1 (ISBN)978-91-8048-413-8 (ISBN)
Public defence
2023-12-14, E632, Luleå tekniska universitet, Luleå, 09:00 (English)
Opponent
Supervisors
Available from: 2023-10-18 Created: 2023-10-18 Last updated: 2025-10-21Bibliographically approved

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Gavrić, SnežanaLeonhardt, GüntherÖsterlund, HeléneMarsalek, JiriViklander, Maria

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