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Mechanical characterisation of a structural battery electrolyte
Industrial and Materials Science, Chalmers University of Technology, 41258, Göteborg, Sweden.
Industrial and Materials Science, Chalmers University of Technology, 41258, Göteborg, Sweden; Tecnica e Gestione dei Sistemi Industriali, Universitá degli Studi di Padova, 36100, Vicenza, Italy.
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Material Science. Institute of Technology, Middle Technical University, Baghdad, Iraq.ORCID iD: 0000-0002-6995-2558
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Material Science.ORCID iD: 0000-0002-5210-4341
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2024 (English)In: Polymer, ISSN 0032-3861, E-ISSN 1873-2291, Vol. 312, article id 127646Article in journal (Refereed) Published
Abstract [en]

Structural battery composites require a structural electrolyte to work. The structural battery electrolyte has a bicontinuous microstructure which enables its dual roles: mechanical load transfer and ion transport between the electrodes. These structural electrolytes are difficult to characterise mechanically via bulk tests. For this reason, no extensive characterisation of the mechanical properties of the structural battery electrolyte has been performed to date. In this study, we highlight the many challenges of these types of tests, including the complexity of sample manufacturing, preparation and testing. We further demonstrate a method to prepare test samples and to perform mechanical tests on the structural battery electrolyte. The executed test campaign provides measures of Young's modulus (approximately 412 MPa) and Poisson's ratio (0.34), as well as tensile (4.85 MPa) and compressive strength (32.66 MPa) and strain to failure (2.49 % and 28.11 % in tension and compression, respectively). In addition, cure shrinkage is investigated and found insignificant. These results are crucial for the further development of structural battery composites as they allow for accurate prediction of their internal stress states.

Place, publisher, year, edition, pages
Elsevier Ltd , 2024. Vol. 312, article id 127646
Keywords [en]
Multifunctionality, Mechanical characterisation, Structural battery electrolyte
National Category
Materials Chemistry
Research subject
Polymeric Composite Materials
Identifiers
URN: urn:nbn:se:ltu:diva-110160DOI: 10.1016/j.polymer.2024.127646ISI: 001322179600001Scopus ID: 2-s2.0-85204366386OAI: oai:DiVA.org:ltu-110160DiVA, id: diva2:1902423
Funder
Vinnova, (Ref. 2019-00068)
Note

Validerad;2024;Nivå 2;2024-10-01 (joosat);

Funder: ONR (USA), (No. N62909-22-1-2037); USAF (USA) EOARD (No. FA8655-21-1-7038);

Full text: CC BY license

Available from: 2024-10-01 Created: 2024-10-01 Last updated: 2025-10-21Bibliographically approved

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Al-Ramahi, NawresJoffe, Roberts

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