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The impact of thermal treatment parameters on the preservation of carbon fiber mechanical properties after reclamation
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Material Science.ORCID iD: 0009-0000-1387-4047
Luleå University of Technology, Department of Engineering Sciences and Mathematics, Energy Science.ORCID iD: 0000-0001-6081-5736
Riga Technical University, Faculty of Natural Sciences and Technology, Institute of Chemistry and Chemical Technology, Paula Valdena iela 3-7, Kurzemes rajons, Rīga, LV-1048, Latvia.
Riga Technical University, Faculty of Natural Sciences and Technology, Institute of Chemistry and Chemical Technology, Paula Valdena iela 3-7, Kurzemes rajons, Rīga, LV-1048, Latvia.
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2024 (English)In: Current Research in Green and Sustainable Chemistry, E-ISSN 2666-0865, Vol. 9, article id 100431Article in journal (Refereed) Published
Abstract [en]

Carbon fiber, despite its exceptional properties, remains underutilized due to monetary and environmental concerns. Concurrently, the imminent challenge associated with rising quantities of End-of-Life CFRP (carbon fiber reinforced polymer) demands the further development of recycling strategies. This study focuses on optimizing the recycling process parameters of pyrolysis and oxidation thermal treatment to maximize the retention of mechanical properties in the recycled fibers in the shortest process time. To assess the result of the pyrolysis, single fiber tensile tests were executed to measure strength and stiffness. Additionally, microscopy and spectroscopy studies were carried out to evaluate fiber geometry as well as surface quality. At the laboratory scale, experiments demonstrated that the combination of pyrolysis and oxidation yields clean, reusable fibers with mechanical properties suitable for secondary applications. The influence of various treatment parameters on the strength and stiffness of the recycled fibers was explored, establishing a clear correlation. The outcome is a set of optimized parameters that contribute to mechanical property retention, including a novel recycling method that allows for reduced processing times, as short as 10 min. This work paves the way for a more eco-friendly and cost-effective approach to harnessing the potential of carbon fiber in a wide range of applications while mitigating environmental concerns associated with landfill disposal.

Place, publisher, year, edition, pages
Elsevier B.V. , 2024. Vol. 9, article id 100431
Keywords [en]
Pyrolysis, Carbon fiber, Composite recycling, CFRP, Polymer composites, Sustainability
National Category
Materials Engineering Chemical Engineering
Research subject
Polymeric Composite Materials; Energy Engineering; Experimental Physics
Identifiers
URN: urn:nbn:se:ltu:diva-110652DOI: 10.1016/j.crgsc.2024.100431Scopus ID: 2-s2.0-85207274252OAI: oai:DiVA.org:ltu-110652DiVA, id: diva2:1910936
Note

Validerad;2024;Nivå 1;2024-11-26 (sarsun);

Full text license: CC BY 4.0;

Available from: 2024-11-06 Created: 2024-11-06 Last updated: 2025-10-21Bibliographically approved

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Corvo Alguacil, MarinaUmeki, KentaroYou, ShujieJoffe, Roberts

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