Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Building surface materials as potential sources of biocides: Insights from laboratory leaching investigations of different material types
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0002-3518-1273
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0002-4732-7348
Luleå University of Technology, Department of Civil, Environmental and Natural Resources Engineering, Architecture and Water.ORCID iD: 0000-0003-1725-6478
2024 (English)In: Chemosphere, ISSN 0045-6535, E-ISSN 1879-1298, Vol. 368, article id 143741Article in journal (Refereed) Published
Abstract [en]

Biocides are incorporated into building surface materials to protect them against algae and fungi growth. When such treated surfaces are exposed to precipitation, they may release these biocides, contaminating receiving water bodies. To regulate the use of biocidal products in line with the European Biocidal Products Regulation it is crucial to identify the precise origin of this type of pollutant. In this study, the leaching of a wide range of biocides and chemical elements from 15 materials was investigated through a laboratory scale experiment. The experimental setup was based on the standard method, SIS-CEN/TS 16637-2:2015. The materials tested included bitumen roofing felt and shingles, impregnated wood, as well as paints intended for concrete, wood, and metal surfaces. Each material was tested in duplicates. All materials were tested at a liquid volume to surface area ratio (L/A) of 22.5 L/m2. Sampling was carried out at three intervals: 6 h, 18 h, and 5 days with the leachant being renewed after each leaching step. The results were that diuron was the most commonly detected biocide from the materials tested. The largest number of biocides, including diuron and its degradation products 1-(3.4-dichlorophenyl) urea (DCPU) and diuron desdimethyl (DCPMU), terbutryn, carbendazim and monuron, were detected in the wood paints. Diuron was detected in all three types of wood paint with a mean areal release ratio of 64.6, 25800, and 5710 μg/m2 for the respective paints. Copper was detected in all leachates from impregnated wood, with mean concentrations of 687, 648, 1450, and 279 μg/L from the four tested wood types, respectively. Some of the biocides released were not reported on the data sheets of the tested materials, indicating a need to investigate broader than only based on the information provided by the manufacturers. Future use of biocides in building surface materials may change due to regulations, phase outs and introduction of new biocides, indicating that source identifications is a continuing effort.

Place, publisher, year, edition, pages
Elsevier, 2024. Vol. 368, article id 143741
Keywords [en]
Stormwater quality, Urban diffuse pollution, Building runoff, DiuronCopper
National Category
Environmental Sciences Other Environmental Engineering
Research subject
Urban Water Engineering; Centre - Centre for Stormwater Management (DRIZZLE)
Identifiers
URN: urn:nbn:se:ltu:diva-110752DOI: 10.1016/j.chemosphere.2024.143741PubMedID: 39542369Scopus ID: 2-s2.0-85208923321OAI: oai:DiVA.org:ltu-110752DiVA, id: diva2:1914201
Funder
Swedish Environmental Protection Agency, NV-05936-22Vinnova, 2022-03092
Note

Validerad;2024;Nivå 1;2024-11-18 (hanlid);

Full text license: CC BY

Available from: 2024-11-18 Created: 2024-11-18 Last updated: 2024-12-12Bibliographically approved

Open Access in DiVA

fulltext(3939 kB)54 downloads
File information
File name FULLTEXT01.pdfFile size 3939 kBChecksum SHA-512
ee7dc6fe2e095b0fe33cce8c6b8ebaa816f68d731b3e7a449a39033bd07b043cf69044287b87a33c844811605c86cd4bce34df629674041534c6734a38b5483e
Type fulltextMimetype application/pdf

Other links

Publisher's full textPubMedScopus

Authority records

Kohzadi, ShadiMüller, AlexandraÖsterlund, HeleneViklander, Maria

Search in DiVA

By author/editor
Kohzadi, ShadiMüller, AlexandraÖsterlund, HeleneViklander, Maria
By organisation
Architecture and Water
In the same journal
Chemosphere
Environmental SciencesOther Environmental Engineering

Search outside of DiVA

GoogleGoogle Scholar
Total: 54 downloads
The number of downloads is the sum of all downloads of full texts. It may include eg previous versions that are now no longer available

doi
pubmed
urn-nbn

Altmetric score

doi
pubmed
urn-nbn
Total: 223 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf